heterogeneous catalysis in organic chemistry(有機化學多相催化)

heterogeneous catalysis in organic chemistry(有機化學多相催化)

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大小:8.05 MB

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時間:2019-01-08

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1、HeterogeneousCatalysisinOrganicChemistryElsevier,2000Author(s):GerardV.SmithandFerencNotheiszISBN:978-0-12-651645-6Preface,Pagesxiii-xvChapter1-IntroductiontoCatalysis,Pages1-28Chapter2-Hydrogenations,Pages29-96Chapter3-EnantioselectiveHydrogenations,Pages97-117Chapter4-Hydro

2、genolysis,Pages119-218Chapter5-BondBreakingReactions,Pages219-227Chapter6-Oxidations,Pages229-246Chapter7-ImmobilizedHomogeneousCatalysts,Pages247-289Appendix,Pages291-293AuthorIndex,Pages295-328SubjectIndex,Pages329-3463040

3、FMPagexiiiThursday,April15,19995:46PMPREFACETheprim

4、aryaimofthisbookistohelptheexperimentalorganicchemistwithheterogeneouscatalyticmethodsformakingandbreakingbonds.Thisbookhastwointentions.First,itisintendedtoservethegraduatestudentsinorganicchemistrywhoneedtoroundouttheireducationandlearnabouthet-erogeneouscatalysisandthemech

5、anismsoforganicreactionsonsurfaces.Second,itisintendedtoaidthebrightorganicchemistswhohavepreparedthenextcompoundthatwillgreatlyimprovethepositionoftheircompanybutwhohavejustbeeninformedbytheirsupervisorsthattheymustmaketheirsyntheticstepsintoheterogeneouscatalyticsteps.Thene

6、edtodemystifyheterogeneousorganicreactionmechanismsisvital.Innoother?eldoforganicchemistryarethereactionscloudedwithfolklore.Nowhereisthereagreaterneedtoclarifya?eldthatisgraduallycomingoutofitsempiricalageandintoitsscienti?cage.Butbarriersexist.Onebarrieristhestartlinglackof

7、anyrequirementsbymanyjournaleditorstopublishchar-acterizationinformationaboutthecatalystsusedinsyntheticpreparations.Thisneedisignoredinspiteofwell-documentedfactsthatthestructureofthecatalystanditspreparationandhistoryin?uenceitsactivityandselectivity.Notrequiringsuchinforma

8、tionpropagatestheideathatthecatalystisa“blackbox”aboutwhichweknownothing.Infact,withoutsuchinformation,itisimpossibletodrawcompletemechanisticconclusionsaboutsurfacereactions;consequently,partofthevalueofpublishedexperimentalsynthesesisirre-trievablylost.Anotherbarrierisuninf

9、ormedandlazyacademicianswhohavelabeledthis?eld“blackmagic,”somanybri

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